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  • Journal article
    Ewers RM, Cook J, Daniel OZ, Orme CDL, Groner V, Joshi J, Rallings A, Rallings T, Amarasekare Pet al., 2024,

    New insights to be gained from a Virtual Ecosystem

    , Ecological Modelling, Vol: 498, ISSN: 0304-3800

    The myriad interactions among individual plants, animals, microbes and their abiotic environment generate emergent phenomena that will determine the future of life on Earth. Here, we argue that holistic ecosystem models – incorporating key biological domains and feedbacks between biotic and abiotic processes and capable of predicting emergent phenomena – are required if we are to understand the functioning of complex, terrestrial ecosystems in a rapidly changing planet. We argue that holistic ecosystem models will provide a framework for integrating the many approaches used to study ecosystems, including biodiversity science, population and community ecology, soil science, biogeochemistry, hydrology and climate science. Holistic models will provide new insights into the nature and importance of feedbacks that cut across scales of space and time, and that connect ecosystem domains such as microbes with animals or above with below ground. They will allow us to critically examine the origins and maintenance of ecosystem stability, resilience and sustainability through the lens of systems theory, and provide a much-needed boost for conservation and the management of natural environments. We outline our approach to developing a holistic ecosystem model – the Virtual Ecosystem – and argue that while the construction of such complex models is obviously ambitious, it is both feasible and necessary.

  • Journal article
    Schroeder AK, Woodward H, Le Cornec CMA, Proust T, Benie PJ, Fan S, Aristodemou E, Jones RL, Linden PF, de Nazelle A, Boies AM, Stettler MEJet al., 2024,

    Vehicle emission models alone are not sufficient to understand full impact of change in traffic signal timings

    , Atmospheric Environment: X, Vol: 24

    Few studies have considered the real-world impact of changes in traffic signal timings on air pollution and pedestrian exposure with most only drawing their conclusion from vehicle emission models alone. Here, we consider two distinct cycle timings at a junction in London, UK, model the impact using a traffic microsimulation and a NOx emissions model, and compare these results with NOx and other air pollution measurements collected during a two-week field study at the junction. Our models predict that extending the cycle time leads to a 23% decrease in NOx emissions within a 15 m radius of the junction itself. When the wind direction was such that our sensors were downwind of the junction a 21% decrease in traffic and background-adjusted NOx concentrations were seen, suggesting that the intervention was successful. However, when the sensors were upwind of the junction, we observed an increase of 23% in adjusted NOx concentrations. Similar patterns were found for the other pollutants NO2, lung deposited surface area, black carbon and CO2 we measured. This indicates that meteorology was by far the greatest determinant of roadside concentrations during our two-week study period. Looking at pedestrian exposure for pedestrians waiting to cross the road, we found that their NOx exposure increased by 46% as waiting times to cross the road increased and that potential small reductions in air pollution were offset by increases in waiting times on the main road. The study demonstrates the need to go beyond assessing the impact of hyper-local traffic interventions on vehicle emissions. Real-world trials over extended periods are required to evaluate the impact of meteorology and changes to air pollution concentrations and pedestrian exposures.

  • Journal article
    Olivelli A, Maxence P, Xu H, Kreissig K, Coles B, Moore R, Bridgestock L, Rijkenberg M, Middag R, Lohan M, Weiss D, Rehkamper M, van de Flierdt Tet al., 2024,

    Vertical transport of anthropogenic lead by reversible scavenging in the South Atlantic Ocean

    , Earth and Planetary Science Letters, Vol: 646, ISSN: 0012-821X

    Stable lead (Pb) isotopes have been regarded as tracers of ocean circulation, both in the present time and geological past. Here we present a new dataset of seawater Pb concentrations and isotope compositions for ten depth profiles from the South Atlantic Ocean (GEOTRACES cruises GA02 and GA10). By comparing Pb isotope data collected on the two cruises, and by modelling the distribution of Pb with an extended optimum multiparameter analysis, we find evidence of vertical transport of anthropogenic Pb pollution due to reversible scavenging. Surface to depth transfer of polluted Pb is aided by high suspended particulate matter loads at the Brazil – Malvinas Confluence and along ∼40°S in the South Atlantic. Overall, our findings caution the use of Pb isotope ratios as ventilation tracers in the South Atlantic and emphasize the importance of particle-seawater interaction for biogeochemical cycles.

  • Journal article
    Blyth L, Graven H, Manning AJ, Levy Pet al., 2024,

    Radiocarbon as a tracer of the fossil fraction of regional carbon monoxide emissions

    , Environmental Research Letters, Vol: 19, Pages: 114073-114073

    <jats:title>Abstract</jats:title> <jats:p>Carbon monoxide (CO) is an atmospheric pollutant with a positive net warming effect on the climate. The magnitude of CO sources and the fraction of fossil vs biogenic sources are still uncertain and vary across emissions inventories. Measurements of radiocarbon (<jats:sup>14</jats:sup>C) in CO could potentially be used to investigate the sources of CO on a regional scale because fossil sources lack <jats:sup>14</jats:sup>C and reduce the <jats:sup>14</jats:sup>C/C ratio (Δ<jats:sup>14</jats:sup>C) of atmospheric CO more than biogenic sources. We use regional Lagrangian model simulations to investigate the utility of Δ<jats:sup>14</jats:sup>CO measurements for estimating the fossil fraction of CO emissions and evaluating bottom-up emissions estimates (United Kingdom Greenhouse Gas, UKGHG, and TNO Copernicus Atmosphere Monitoring Service, TNO) in London, UK. Due to the high Δ<jats:sup>14</jats:sup>CO in atmospheric CO from cosmogenic production, both fossil and biogenic CO emissions cause large reductions in Δ<jats:sup>14</jats:sup>CO regionally, with larger reductions for fossil than biogenic CO per ppb added. There is a strong seasonal variation in Δ<jats:sup>14</jats:sup>CO in background air and in the sensitivity of Δ<jats:sup>14</jats:sup>CO to fossil and biogenic emissions of CO. In the UK, the CO emissions estimate from TNO has a higher fraction from fossil fuels than UKGHG (72% vs 67%). This results in larger simulated decreases in Δ<jats:sup>14</jats:sup>C per ppb CO for TNO emissions. The simulated differences between UKGHG and TNO are likely to be easily detectable by current measurement precision, suggesting that Δ<jats:sup>14</jats:sup>CO measurements could be an effective tool to understand regional CO so

  • Journal article
    Alonzo D, Tabelin CB, Dalona IM, Abril JMV, Beltran A, Orbecido A, Villacorte-Tabelin M, Resabal VJ, Promentilla MA, Suelto M, Brito-Parada PR, Plancherel Y, Jungblut AD, Armstrong R, Santos A, Schofield PF, Herrington Ret al., 2024,

    Working with the community for the rehabilitation of legacy mines: Approaches and lessons learned from the literature

    , Resources Policy, Vol: 98, ISSN: 0301-4207
  • Journal article
    Saceanu MC, Paluszny A, Ivars DM, Zimmerman RWet al., 2024,

    Thermo-mechanical modelling of spalling around the deposition boreholes in an underground nuclear waste repository during its thermal phase

    , International Journal of Rock Mechanics and Mining Sciences, Vol: 183, ISSN: 1365-1609

    This paper presents a three-dimensional numerical analysis of multiple fracture growth leading to the development of excavation disturbed zones and spalling around deposition boreholes in a geological disposal facility. The development of fracture patterns is simulated with the Imperial College Geomechanics Toolkit, a finite-element based simulator that can model the simultaneous nucleation, growth, and coalescence of multiple fractures in quasi-brittle rock. In these simulations, fractures develop due to the stress concentrations around the borehole wall, caused by the local in situ stresses, and due to the thermal stresses caused by the radioactive decay of the waste. Fracture patterns, and the extent of the spalled zone, are computed after the borehole drilling, heating, and cooling stages, at the Forsmark repository site in Sweden. The effect of temperature on the nucleation and growth of spalling fractures, as well as on the reactivation of pre-existing fractures, is assessed qualitatively, by comparing fracture patterns, and quantitatively, in terms of the maximum spalling depth, width, and increase in the total fractured surface area. Overall, the simulations presented herein indicate that thermal spalling will increase the depths (away from the borehole) and angular widths of the spalled zone, but is not likely to lead to major increases in fracture aperture, and concomitant increases in hydraulic transmissivity and permeability of the spalled zone, above that which has already been caused by mechanical spalling.

  • Journal article
    Dray L, Kuleszo J, Teoh R, Stettler M, Stewart J, Schäfer Aet al., 2024,

    Global air freight flow data for aviation policy modelling

    , Journal of Air Transport Management, Vol: 121, Pages: 102692-102692, ISSN: 0969-6997
  • Journal article
    Ceppi P, Myers TA, Nowack P, Wall CJ, Zelinka MDet al., 2024,

    Implications of a Pervasive Climate Model Bias for Low‐Cloud Feedback

    , Geophysical Research Letters, Vol: 51, ISSN: 0094-8276

    <jats:title>Abstract</jats:title><jats:p>How low clouds respond to warming constitutes a key uncertainty for climate projections. Here we observationally constrain low‐cloud feedback through a controlling factor analysis based on ridge regression. We find a moderately positive global low‐cloud feedback (0.45 W , 90% range 0.18–0.72 W ), about twice the mean value (0.22 W ) of 16 models from the Coupled Model Intercomparison Project. We link this discrepancy to a pervasive model mean‐state bias: models underestimate the low‐cloud response to warming because (a) they systematically underestimate present‐day tropical marine low‐cloud amount, and (b) the low‐cloud sensitivity to warming is proportional to this present‐day low‐cloud amount. Our results hence highlight the importance of reducing model biases in both the mean state of clouds and their sensitivity to environmental factors for accurate climate change projections.</jats:p>

  • Journal article
    Stocker B, Dong N, Perkowski EA, Schneider PD, Xu H, de Boer H, Rebel KT, Smith NG, Van Sundert K, Wang H, Jones SE, Prentice IC, Harrison SPet al., 2024,

    Empirical evidence and theoretical understanding ofecosystem carbon and nitrogen cycle interactions

    , New Phytologist, ISSN: 0028-646X
  • Journal article
    Nathwani C, Blundy J, Large S, Wilkinson J, Buret Y, Loader M, Tavazzani L, Chelle-Michou Cet al., 2024,

    A zircon case for super-wet arc magmas

    , Nature Communications, ISSN: 2041-1723

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